Experimental realization of a polarization-independent ultraviolet/visible coaxial plasmonic metamaterial

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DOI http://dx.doi.org/10.1021/nl5028183
Reference M.A. van de Haar, R.C. Maas, A.H. Schokker and A. Polman, Experimental realization of a polarization-independent ultraviolet/visible coaxial plasmonic metamaterial, Nano Lett. 14, (11), 6356-6360 (2014)
Group Photonic Materials

We report the experimental realization of an optical metamaterial composed of a hexagonal array of coaxial plasmonic metal/insulator/metal waveguides that shows strong polarization-independent optical mode index dispersion in the ultraviolet/blue. The metamaterial is composed of silicon coaxes with a well-defined diameter in the range of 150-168 nm with extremely thin sidewalls (13-15 nm), embedded in a silver film, fabricated using a combination of electron beam lithography, physical vapor deposition, reactive ion etching, and focused ion beam polishing. Using a Mach-Zehnder interferometer the phase advance is measured on several metamaterial samples with different dimensions in the UV/visible part of the spectrum. For all geometries the spectral features as well as the geometry dependence of the data correspond well with numerical finite-difference time domain simulations and the calculated waveguide dispersion diagram, showing a negative mode index between 440 and 500 nm.